Prior to the live performance of "Crazy" for Gnarls Barkley, Cat Power, the stage name of Chan Marshall, had released her album "The Greatest" in 2006, a significant work that marked a turning point in her career. This album was noted for its soulful sound and included collaborations with renowned musicians. At this time, Marshall was gaining recognition for her distinct artistic voice and evocative songwriting, which would be showcased in her live rendition of "Crazy." Interestingly, the performance reflects her ability to reinterpret songs through her unique style, demonstrating her versatility as an artist. Following "The Greatest," she would explore various genres and continue to evolve her sound, further solidifying her place in the music industry. The live recording highlights her emotional delivery and connection to the audience, characteristics that define her career.