The live performance of "Dirty Harry" at the BRIT Awards took place in 2006, during a notable period in Gorillaz's career following the release of their second studio album, "Demon Days" (2005). This album marked a significant evolution in their sound and featured several hit singles, including "Feel Good Inc." and "Dirty Harry." By this time, Gorillaz had established themselves as a groundbreaking virtual band, blending animated visuals with diverse musical styles. The BRITs performance was particularly interesting as it showcased their innovative approach to live shows, incorporating animated elements alongside live musicians and guest appearances. This blend of multimedia presence was emblematic of their unique identity, further solidifying their place in popular music during the mid-2000s.